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Abstract:

Recent scanning tunneling microscopy experiments in twisted bilayer [K. P. Nuckolls et al., Nature (London) 620, 525 (2023)] and trilayer [H. Kim et al., Nature (London) 623, 942 (2023)] graphene have revealed the ubiquity of Kekulé charge-density wave order in magic-angle graphene. Most samples are moderately strained and show “incommensurate Kekulé spiral” (IKS) order involving a graphene-scale charge density distortion uniaxially modulated on the scale of the moiré superlattice, in accord with theoretical predictions. However, ultralow strain bilayer samples instead show graphene-scale Kekulé charge order that is uniform on the moiré scale. This order, especially prominent near filling factor 𝜈=−2, is unanticipated by theory which predicts a time-reversal breaking Kekulé current order at low strain. We show that including the coupling of moiré electrons to graphene-scale optical zone-corner (ZC) phonons stabilizes a uniform Kekulé charge ordered state at |𝜈|=2 with a quantized topological (spin or anomalous Hall) response. Our work clarifies how this phonon-driven selection of electronic order emerges in the strong-coupling regime of moiré graphene.