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Abstract:

Context. Growing evidence has indicated that the global composition distribution plays an indisputable role in interpreting observational data. Three-dimensional general circulation models (GCMs) with a reliable treatment of chemistry and clouds are particularly crucial in preparing for upcoming observations. In attempts to achieve 3D chemistry-climate modeling, the challenge mainly lies in the expensive computing power required for treating a large number of chemical species and reactions.
Aims. Motivated by the need for a robust and computationally efficient chemical scheme, we devise a mini-chemical network with a minimal number of species and reactions for H2-dominated atmospheres.
Methods. We apply a novel technique to simplify the chemical network from a full kinetics model, VULCAN, by replacing a large number of intermediate reactions with net reactions. The number of chemical species is cut down from 67 to 12, with the major species of thermal and observational importance retained, including H2O, CH4, CO, CO2, C2H2, NH3, and HCN. The size of the total reactions is also greatly reduced, from ~800 to 20. We validated the mini-chemical scheme by verifying the temporal evolution and benchmarking the predicted compositions in four exoplanet atmospheres (GJ 1214b, GJ 436b, HD 189733b, and HD 209458b) against the full kinetics of VULCAN.
Results. The mini-network reproduces the chemical timescales and composition distributions of the full kinetics well within an order of magnitude for the major species in the pressure range of 1 bar–0.1 mbar across various metallicities and carbon-to-oxygen (C/O) ratios.
Conclusions. We have developed and validated a mini-chemical scheme using net reactions to significantly simplify a large chemical network. The small scale of the mini-chemical scheme permits simple use and fast computation, which is optimal for implementation in a 3D GCM or a retrieval framework. We focus on the thermochemical kinetics of net reactions in this paper and address photochemistry in a follow-up paper.

Abstract:

In the tropical stratosphere, deep layers of eastward and westward winds encircle the globe and descend regularly from the upper stratosphere to the tropical tropopause. With a complete cycle typically lasting almost 2.5 years, this quasi-biennial oscillation (QBO) is arguably the most predictable mode of atmospheric variability that is not linked to the changing seasons. The QBO affects climate phenomena outside the tropical stratosphere, including ozone transport, the North Atlantic Oscillation and the Madden–Julian Oscillation, and its high predictability could enable better forecasts of these phenomena if models can accurately represent the coupling processes. Climate and forecasting models are increasingly able to simulate stratospheric oscillations resembling the QBO, but exhibit common systematic errors such as weak amplitude in the lowermost tropical stratosphere. Uncertainties about the waves that force the oscillation, particularly the momentum fluxes from small-scale gravity waves excited by deep convection, make its simulation challenging. Improved representation of the processes governing the QBO is expected to lead to better forecasts of the oscillation and its impacts, increased understanding of unusual events such as the two QBO disruptions observed since 2016, and more reliable future projections of QBO behaviour under climate change.

Abstract:

The influence of the quasi-biennial oscillation (QBO) on tropical climate is demonstrated using 500-year pre-industrial control simulations from the Met Office Hadley Centre model. Robust precipitation responses to the phase of the QBO are diagnosed in the model, which show zonally asymmetric patterns that resemble the El Niño–Southern Oscillation (ENSO) impacts. These patterns are found because the frequency of ENSO events for each QBO phase is significantly different in these simulations, with more El Niño events found under the westerly phase of the QBO (QBOW) and more La Niña events for the easterly phase (QBOE). The QBO–ENSO relationship is non-stationary and subject to decadal variability in both models and observations. In addition, regression analysis shows that there is a QBO signal in precipitation that is independent of ENSO. No evidence is found to suggest that these QBO–ENSO relationships are caused by ENSO modulating the QBO in the simulations. A relationship between the QBO and a dipole of precipitation in the Indian Ocean is also found in models and observations in boreal fall, characterised by a wetter western Indian Ocean and drier conditions in the eastern part for QBOW and the opposite under QBOE conditions. The Walker circulation is significantly weaker during QBOW compared to QBOE, which could explain the observed and simulated zonally asymmetric precipitation responses at equatorial latitudes, as well as the more frequent El Niño events during QBOW. Further work, including targeted model experiments, is required to better understand the mechanisms causing these relationships between the QBO and tropical convection.

Abstract:

The January 2022 Hunga Tonga–Hunga Haʻapai eruption was one of the most explosive volcanic events of the modern era^1,2, producing a vertical plume which peaked > 50km above the Earth³. The initial explosion and subsequent plume triggered atmospheric waves which propagated around the world multiple times⁴. A global-scale wave response of this magnitude from a single source has not previously been observed. Here we show the details of this response, using a comprehensive set of satellite and ground-based observations to quantify it from surface to ionosphere. A broad spectrum of waves was triggered by the initial explosion, including Lamb waves^5,6 propagating at phase speeds of 318.2±6 ms^-1 at surface level and between 308±5 to 319±4 ms^-1 in the stratosphere, and gravity waves⁷ propagating at 238±3 to 269±3 ms^-1 in the stratosphere. Gravity waves at sub-ionospheric heights have not previously been observed propagating at this speed or over the whole Earth from a single source^8,9. Latent heat release from the plume remained the most significant individual gravity wave source worldwide for >12 hours, producing circular wavefronts visible across the Pacific basin in satellite observations. A single source dominating such a large region is also unique in the observational record. The Hunga Tonga eruption represents a key natural experiment in how the atmosphere responds to a sudden point-source-driven state change, which will be of use for improving weather and climate models.

Abstract:

Lava planets have non-global, condensible atmospheres similar to icy bodies within the Solar system. Because they depend on interior dynamics, studying the atmospheres of lava planets can lead to understanding unique geological processes driven by their extreme environment. Models of lava planet atmospheres have thus far focused on either radiative transfer or hydrodynamics. In this study, we couple the two processes by introducing ultraviolet (UV) and infrared (IR) radiation to a turbulent boundary layer model. We also test the effect of different vertical temperature profiles on atmospheric dynamics. Results from the model show that UV radiation affects the atmosphere much more than IR. UV heating and cooling work together to produce a horizontally isothermal atmosphere away from the substellar point regardless of the vertical temperature profile. We also find that stronger temperature inversions induce stronger winds and hence cool the atmosphere. Our simulated transmission spectra of the bound atmosphere show a strong SiO feature in the UV that would be challenging to observe in the planet’s transit spectrum due to the precision required. Our simulated emission spectra are more promising, with significant SiO spectral features at 4.5 and 9 μm that can be observed with the James Webb Space Telescope. Different vertical temperature profiles produce discernible dayside emission spectra, but not in the way one would expect.